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The kinetics of the reactions of C2H radical with ethane (k1), propane (k2), and n-butane (k3) are studied over the temperature range of T = 96-296 K with a pulsed Laval nozzle apparatus that utilizes a pulsed laser photolysis-chemiluminescence technique. The C2H decay profiles in the presence of both the alkane reactant and O2 are monitored by the CH(A2Δ) chemiluminescence tracer method. The results, together with available literature data, yield the following Arrhenius expressions: k1(T) = (0.51 ± 0.06) × 10−10 exp[(−76 ± 30)K/T] cm3 molecule−1 s−1 (T = 96-800 K), k2(T) = (0.98 ± 0.32) × 10−10exp[(−71 ± 60)K/T] cm3 molecule−1 s−1 (T = 96-361 K), and k3(T) = (1.23 ± 0.26) × 10−10 cm3 molecule−1 s−1 (T = 96-297 K). At T = 296 K, k1 is measured as a function of total pressure and has little or no pressure dependence. The results from this work support a direct hydrogen abstraction mechanism for the title reactions. Implications to the atmospheric chemistry of Titan are discussed. 相似文献
23.
Mars Global Surveyor accelerometer observations of the martian upper atmosphere revealed large variations in density with longitude during northern hemisphere spring at altitudes of 130-160 km, all latitudes, and mid-afternoon local solar times (LSTs). This zonal structure is due to tides from the surface. The zonal structure is stable on timescales of weeks, decays with increasing altitude above 130 km, and is dominated by wave-3 (average amplitude 22% of mean density) and wave-2 (18%) harmonics. The phases of these harmonics are constant with both altitude and latitude, though their amplitudes change significantly with latitude. Near the South Pole, the phase of the wave-2 harmonic changes by 90° with a change of half a martian solar day while the wave-3 phase stays constant, suggesting diurnal and semidiurnal behaviour, respectively. We use a simple application of classical tidal theory to identify the dominant tidal modes and obtain results consistent with those of General Circulation Models. Our method is less rigorous, but simpler, than the General Circulation Models and hence complements them. Topography has a strong influence on the zonal structure. 相似文献
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本文简要介绍了陆地系列地球资源卫星的轨道特征,并以陆地—5号资源卫星为例,根据南山站的座标计算出该站对陆地—5号资源卫星的可观测范围及以该站为中心的卫星的覆盖区域。 相似文献
26.
Mercury (Hg) was investigated in bone tissues of skua ( Catharacta maccormick) and penguin (Pygoscelis adeliae) collected in the maritime Antarctic using atomic fluorescence spectrometry (AFS) and synchrotron radiation X-ray fluorescence (SR-XRF) method. The total levels of mercury in bone tissues of penguin and skua are much lower than those in other organs (e. g. , kidney, liver). The toxic effects of mercury in bone tissues of seabirds in polar region are not known. We have used SR- XRF method to map the distribution of trace levels of mercury in bones. The levels of mercury are found to be enriched somewhere near the periosteal surface and/or endosteal surface. The distribution of mercury shows strongly correlation with that of some essential elements and probably poses negative effect on the bone metabolism inferring from the relationship of mercury with the other elements. These studies represent a first step toward understanding the toxic effects of mercury on bone of polar animals by suggesting the possible microscopic investigation. 相似文献
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广西海洋资源丰富 ,品种繁多 ,为了更好开发 ,建议从法制、宣传教育、普及海洋资源有关知识 ,提高人们整体素质做起 ,进一步抓住机遇 ,合理开发 ,才能取得良好效益 ,达到预定目标 相似文献
30.
Calibrating the GOCE accelerations with star sensor data and a global gravity field model 总被引:1,自引:0,他引:1
A reliable and accurate gradiometer calibration is essential for the scientific return of the gravity field and steady-state
ocean circulation explorer (GOCE) mission. This paper describes a new method for external calibration of the GOCE gradiometer
accelerations. A global gravity field model in combination with star sensor quaternions is used to compute reference differential
accelerations, which may be used to estimate various combinations of gradiometer scale factors, internal gradiometer misalignments
and misalignments between star sensor and gradiometer. In many aspects, the new method is complementary to the GOCE in-flight
calibration. In contrast to the in-flight calibration, which requires a satellite-shaking phase, the new method uses data
from the nominal measurement phases. The results of a simulation study show that gradiometer scale factors can be estimated
on a weekly basis with accuracies better than 2 × 10−3 for the ultrasensitive and 10−2 for the less sensitive axes, which is compatible with the requirements of the gravity gradient error. Based on a 58-day data
set, scale factors are found that can reduce the errors of the in-flight-calibrated measurements. The elements of the complete
inverse calibration matrix, representing both the internal gradiometer misalignments and scale factors, can be estimated with
accuracies in general better than 10−3. 相似文献